Personally, I'm most surprised by #16, an anime that I had barely heard of apparently beating out K-On! at its own game, and #12, Joker Game, which didn't leave much of an impression when I watched it.
The Translated list:
81~100: 100 - tatami galaxy
99 - Gan to Gon
98 - Macross Do You Remember Love
97 - Akira
96 - jojo stardust
95 - denou coil
94 - Urusei Yatsura 2 Beautiful Dreamer
93 - inuyasha
92 - kill la kill
91 - mononoke (not princess)
90 - nadia
89 - hetalia beautiful world
88 - kekkai sensen
87 - The Twelve Kingdoms
86 - Armored Trooper Votoms
85 - pokemon
84 - HxH (original)
83 - anohana
82 - kuroko no basket s1
81 - K
71~80:
80: Rakugo Shinjuu
79: Urusei yatsura
78: Mushishi
77: Angel Beats!
76: Cardcaptor Sakura2
75: Space Battleship Yamato Warriors of Love
74: Shonen Hollywood
73: MacrossF
72: One Piece
71: FMA
51~70:
70: Gundam Iron Blooded Orphan
69: Mob Psycho 100
68: GochiUsa2
67: Haikyuu Second Season
66: The IDOLM@STER
65: Yuyu Hakushou
64: Hitman Reborn
63: Free! Starting Days
62: Free Eternal Summer
61: Re:zero
60: Sailor Moon
59: Castle in the Sky Laputa
58: K-on!!
57: Kimi no Na wa
56: Utapri 1000%
55: Gintama'
54: Nausicca
53: Pokemon Diamond & Pearl Movie
52: Shirobako
51: KimiUso
41~50:
50 : Fate Zero
49 - Girls and Panzer Movie
48 - Free
47 - Hibike Euphonium
46 - Ghost in the Shell SAC
45 - Bakemonogatari
44 - Lupin III Cagliostro
43 - TTGL
42 - Haruhi S1
41 - K-on S1
31~40:
40 - Gundam SEED
39 - Future Boy Conan
38 - Hoshi no Ko Poron
37 - F/SN UBW
36 - Natsume Yuujinchou
35 - Steins Gate
34 - Cowboy Bebop
33 - LL Sunshine
32 - Prince of Tennis
31 - Stray Dogs S1
26~30:
30 - Utena
29 - Space Battleship Yamato (original)
28 - Attack on Titan
27 - Fullmetal Alchemist Brotherhood
26 - Madoka Movie 3 Rebellion
21~25:
25 - Hyouka
24 - Detective Conan
23 - Haikyuu
22 - Girls und Panzer
21 - Clannad After Story
16~20:
20 - SAO
19 - Psycho-Pass
18 - Digimon Adventure
17 - Mobile Suit Gundam
16 - GochiUsa
Top 15:
15 - Code Geass R2
14 - eva
13 - legend of galactic heroes
12 - joker game
11 - gintamaSPOILER: Show10 - Osomatsu-san
9 - Love Live Movie
8 - Cardcaptor Sakura
7 - Code geass
6 - Tiger and Bunny: Beginning
5 - Love Live 2
4 - Love Live
3rd place: Madoka Magica
2nd place: Tiger and Bunny: Rising
and
first place
Tiger and Bunny